Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films

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A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä
Date
2023-04
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en
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7
1-7
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Physical Review Materials, Volume 7, issue 4
Abstract
We present a study on the structural and magnetic properties of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2)O3 (Lu5BO) high-entropy oxide perovskite thin films. We use synchrotron-based x-ray absorption spectroscopy employing x-ray magnetic circular and linear dichroism (XMCD and XMLD) to perform an element-sensitive study on single-crystal epitaxial Lu5BO thin films. Together with XMCD magnetometry, the results reveal dominant antiferromagnetic order with a transition temperature around 100 K.
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Funding Information: The authors thank A. Kleibert and Y.-L. Huang for their support and fruitful discussions. This work was supported by the Academy of Finland (Project No. 316857) and part of this work was performed at the XTreme beamline of the Swiss Light Source. F.S. is funded by the Swiss National Science Foundation (SNF) (Grant No. 200021_184684). SQUID-VSM measurements were carried out on the Quantum Design MPMS3-137 device of the Laboratory for Mesoscopic Systems, ETH Zurich, Switzerland and the Laboratory for Multiscale Materials Experiments, Paul Scherrer Institute, Switzerland. We acknowledge the provision of facilities and technical support by Aalto University at OtaNano - Nanomicroscopy Center (Aalto-NMC). Publisher Copyright: © 2023 American Physical Society.
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Farhan, A, Cocconcelli, M, Stramaglia, F, Kuznetsov, N, Flajšman, L, Wyss, M, Yao, L, Piamonteze, C & Van Dijken, S 2023, ' Element-sensitive x-ray absorption spectroscopy and magnetometry of Lu(Fe0.2Mn0.2Co0.2Cr0.2Ni0.2) O3 high-entropy oxide perovskite thin films ', Physical Review Materials, vol. 7, no. 4, 044402, pp. 1-7 . https://doi.org/10.1103/PhysRevMaterials.7.044402