Photochemical Synthesis of Tungsten Pentafluoride, WF5

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A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

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en

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7

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Zeitschrift fur Anorganische und Allgemeine Chemie, Volume 647, issue 4, pp. 218-224

Abstract

A new synthetic route for the synthesis of WF5 utilizing a mercury photosensitized reduction of tungsten hexafluoride with H2 is described. Crystals of WF5 were studied using single-crystal X-ray diffraction, resulting in the first-reported crystal structure of WF5. Powder X-ray diffraction studied at room-temperature showed the compound was phase-pure. The IR spectrum of WF5 was reinvestigated and interpreted with the use of solid-state quantum-chemical calculations using the DFT-PBE0 density functional method. The compound synthesized herein was free of HF and moisture but may have contained minute amounts of WOF4, that were only observed in the IR spectrum.

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Stene, R, Scheibe, B, Ivlev, S I, Karttunen, A J, Petry, W & Kraus, F 2021, 'Photochemical Synthesis of Tungsten Pentafluoride, WF 5', Zeitschrift fur Anorganische und Allgemeine Chemie, vol. 647, no. 4, pp. 218-224. https://doi.org/10.1002/zaac.202000177