First-principles simulation of intrinsic collision cascades in KCl and NaCl to test interatomic potentials at energies between 5 and 350 eV

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© 1991 American Physical Society (APS). This is the accepted version of the following article: Keinonen, J. & Kuronen, A. & Tikkanen, P. & Börner, H. G. & Jolie, J. & Ulbig, S. & Kessler, E. G. & Nieminen, Risto M. & Puska, M. J. & Seitsonen, A. P. 1991. First-principles simulation of intrinsic collision cascades in KCl and NaCl to test interatomic potentials at energies between 5 and 350 eV. Physical Review Letters. Volume 67, Issue 26. 3692-3695. ISSN 0031-9007 (printed). DOI: 10.1103/physrevlett.67.3692, which has been published in final form at http://journals.aps.org/prl/abstract/10.1103/PhysRevLett.67.3692.

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Journal Title

Journal ISSN

Volume Title

School of Science | A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Date

1991

Major/Subject

Mcode

Degree programme

Language

en

Pages

3692-3695

Series

Physical Review Letters, Volume 67, Issue 26

Abstract

Theoretical interatomic potentials for KCl and NaCl are tested at energies 5–350 eV against experimental data from intrinsic collision cascades. The collisional scattering of Cl with Cl, K, and Na atoms was observed from Doppler-shifted γ rays depopulating an excited state in recoiling Cl36 produced through the thermal neutron capture Cl35(n,γ)36Cl. The collisional scattering was simulated with molecular dynamics. Interatomic potentials from the present Iab initioP atomic cluster calculations are proposed for the Cl-Cl, Cl-K, and Cl-Na interactions in KCl and NaCl.

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Keywords

KCl, NaCl, interatomic potentials

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Citation

Keinonen, J. & Kuronen, A. & Tikkanen, P. & Börner, H. G. & Jolie, J. & Ulbig, S. & Kessler, E. G. & Nieminen, Risto M. & Puska, M. J. & Seitsonen, A. P. 1991. First-principles simulation of intrinsic collision cascades in KCl and NaCl to test interatomic potentials at energies between 5 and 350 eV. Physical Review Letters. Volume 67, Issue 26. 3692-3695. ISSN 0031-9007 (printed). DOI: 10.1103/physrevlett.67.3692.