Single- and Multilayers of Alkali Metal Atoms inside Graphene/MoS2Heterostructures: A Systematic First-Principles Study

No Thumbnail Available

Access rights

openAccess

URL

Journal Title

Journal ISSN

Volume Title

A1 Alkuperäisartikkeli tieteellisessä aikakauslehdessä

Date

2022-09-07

Major/Subject

Mcode

Degree programme

Language

en

Pages

15558−15564

Series

Journal of Physical Chemistry C, Volume 126, issue 37

Abstract

Stacking various 2D materials in van der Waals heterostructures is a novel approach to design new systems, which can host alkali metal (AM) atoms to tune their electronic properties or store energy. Using state-of-the-art first-principles calculations, we systematically study the intercalation of the most widespread AMs (Li, Na, and K) into a graphene/MoS2 heterostructure. Contrary to the previous work on the intercalation of AMs into various heterostructures based on 2D materials, we consider not only single-, but also multi-layer configurations of AM atoms. We assess the intercalation energetics for various concentrations of AM atoms, calculate charge transfer from AM atoms to the host system, and show that although intercalation of AMs as a single layer is energetically preferable, multi-layer configurations can exist at high concentrations of AM atoms. We further demonstrate that the transition of the MoS2 layer from the H to T′ phase is possible upon Li intercalation, but not for Na or K. Our findings should help to better understand the behavior of heterostructures upon AM atom intercalation and may stimulate further experiments aimed at the tailoring of heterostructure properties and increasing the capacity of anode materials in AM ion batteries.

Description

Funding Information: We thank Dr. M. Ghorbani-Asl for fruitful discussion. A.V.K. acknowledges the German Research Foundation (DFG) for the support through project KR 4866/6-1 and the collaborative research center “Chemistry of Synthetic 2D Materials” SFB-1415-417590517. J.H.S. acknowledges financial support from the EU graphene flagship core 3 program. I.V.C. thanks the German Academic Exchange Service (DAAD) program “Mikhail Lomonosov” for support. The authors thank the HZDR Computing Center, HLRS, Stuttgart, Germany, and TU Dresden Cluster “Taurus” for generous grants of CPU time. Publisher Copyright: © 2022 American Chemical Society.

Keywords

Other note

Citation

Chepkasov , I V , Smet , J H & Krasheninnikov , A V 2022 , ' Single- and Multilayers of Alkali Metal Atoms inside Graphene/MoS 2 Heterostructures: A Systematic First-Principles Study ' , Journal of Physical Chemistry C , vol. 126 , no. 37 , pp. 15558−15564 . https://doi.org/10.1021/acs.jpcc.2c03749