Nuclear magnetism and superconductivity : investigations on lithium and rhodium

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dc.contributor Aalto-yliopisto fi
dc.contributor Aalto University en
dc.contributor.author Juntunen, Kirsi
dc.date.accessioned 2012-02-17T06:47:00Z
dc.date.available 2012-02-17T06:47:00Z
dc.date.issued 2005-02-19
dc.identifier.isbn 951-22-7487-6
dc.identifier.uri https://aaltodoc.aalto.fi/handle/123456789/2530
dc.description.abstract This thesis describes low temperature experiments on lithium. The experiments concentrate on investigating low temperature phase transitions of two subsystems in this metal: its nuclear spin and electronic systems. These phenomena were investigated in two separate sets of samples, each designed to meet the experimental requirements for the phenomena under investigation. The electronic ground state of lithium at ambient pressures is expected to be superconducting, but earlier experiments show that the metal remains normal at least down to 4 mK. In this thesis research, a lithium sample was cooled down to 0.1 mK, B < 10 nT, but no superconductivity was observed. A new upper limit for the superconducting transition temperature was established, over an order of magnitude lower than the earlier upper limit. Many theoretical estimates predict superconductivity already at higher temperatures, and its absence remains a puzzle. The superconductivity in lithium has been under considerable interest recently, since the superconducting phase was observed in the highly compressed state. The nuclear spin system of lithium was investigated as well. The large magnetic moment of the lithium-7 nuclei made lithium an interesting target for studies of nuclear magnetism. The spin system was cooled down by a two stage adiabatic nuclear demagnetization cryostat. The nuclear magnetic resonance (NMR) spectra, the spin temperature, and the static susceptibility were measured. The NMR spectra revealed the appearance of an anomalous peak at low frequencies. Also, the spin system was found to behave in an irreversible manner at low fields and high nuclear polarizations. These effects give evidence for the existence of a magnetically ordered state of the lithium nuclei. The type of the order was not resolved unambiguously, but some facts point to a ferromagnetic ordering. A tentative phase diagram was constructed for the system. Previously, nuclear magnetism and superconductivity in rhodium metal have been investigated. This thesis also includes some numerical and analytical modeling on the nuclear spin system of rhodium, aimed at the interpretation of the experimental data. en
dc.format.extent 42, [154]
dc.format.mimetype application/pdf
dc.language.iso en en
dc.publisher Helsinki University of Technology en
dc.publisher Teknillinen korkeakoulu fi
dc.relation.haspart T. A. Knuuttila, J. T. Tuoriniemi, K. Lefmann, K. I. Juntunen, F. B. Rasmussen, and K. K. Nummila. 2001. Polarized nuclei in normal and superconducting rhodium. Journal of Low Temperature Physics 123, numbers 1-2, pages 65-102.
dc.relation.haspart K. I. Juntunen, K. Lefmann, J. T. Tuoriniemi, and T. A. Knuuttila. 2001. High temperature expansion and exact diagonalization of the rhodium nuclear spin system compared to experimental results. Journal of Low Temperature Physics 124, pages 271-289. [article2.pdf] © 2001 by authors and © 2001 Springer Science+Business Media. By permission.
dc.relation.haspart J. T. Tuoriniemi, K. I. Juntunen, and J. M. Uusvuori. 2003. Thermal contact to lithium metal. Physica B 329-333, pages 1294-1295. [article3.pdf] © 2003 Elsevier Science. By permission.
dc.relation.haspart J. T. Tuoriniemi and K. I. Juntunen. 2004. Nuclei in cooperation. Journal of Low Temperature Physics 135, pages 513-543. [article4.pdf] © 2004 by authors and © 2004 Springer Science+Business Media. By permission.
dc.relation.haspart K. I. Juntunen and J. T. Tuoriniemi. 2005. NMR spectra of highly polarized lithium. Journal of Low Temperature Physics 138, pages 759-764. [article5.pdf] © 2005 by authors and © 2005 Springer Science+Business Media. By permission.
dc.relation.haspart K. I. Juntunen and J. T. Tuoriniemi. 2004. Nuclear ordering in lithium and an upper limit on its ambient pressure superconducting transition temperature. Physical Review Letters 93, number 15, 157201 : pages 1-4. [article6.pdf] © 2004 American Physical Society. By permission.
dc.relation.haspart K. I. Juntunen and J. T. Tuoriniemi. 2004. Experiment on nuclear ordering and superconductivity in lithium. Helsinki University of Technology, Low Temperature Laboratory publications, Report 12 (TKK-KYL-012). 52 pages. [article7.pdf] © 2004 by authors.
dc.subject.other Physics en
dc.title Nuclear magnetism and superconductivity : investigations on lithium and rhodium en
dc.type G5 Artikkeliväitöskirja fi
dc.description.version reviewed en
dc.contributor.department Department of Engineering Physics and Mathematics en
dc.contributor.department Teknillisen fysiikan ja matematiikan osasto fi
dc.subject.keyword lithium en
dc.subject.keyword rhodium en
dc.subject.keyword ultralow temperatures en
dc.subject.keyword nuclear magnetic ordering en
dc.subject.keyword nuclear magnetism en
dc.subject.keyword superconductivity en
dc.identifier.urn urn:nbn:fi:tkk-004781
dc.type.dcmitype text en
dc.type.ontasot Väitöskirja (artikkeli) fi
dc.type.ontasot Doctoral dissertation (article-based) en
dc.contributor.lab Low Temperature Laboratory en
dc.contributor.lab Kylmälaboratorio fi


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